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1 Introduction 1.1 Look Back on Optical Digital Data Storage 1.1.1 Progress of Digital Data Storage 1.1.2 From VCD to Blu-Ray Disc 1.2 Research and Development of Optical Storage in China 1.2.1 Multi-wavelength and Multilevel Storage 1.2.2 Volume Holographic Storage 1.2.3 Near-Field Optical Storage 1.2.4 Big Data Storage System Integration 1.2.5 New Storage Materials and Medium 1.2.6 Chinese Blue High Density Disc 1.3 The Advanced Efforts for Multi-dimension Optical Storage 1.3.1 3-Dimension (3D) Optical Storage 1.3.2 5-Dimensional Optical Storage 1.3.3 Negative Refraction Index Materials Application to SIL 3-Dimensional Storage 1.3.4 The Higher Order Radially Polarized Beams Application in SIL 1.3.5 Other Schemes for Multi-value Optical Storage 1.4 Frontier Science and Technologies Related to Optical Storage.. 1.4.1 Ultraviolet Optical Storage 1.4.2 Plasmonic Optical Storage 1.4.3 X-Ray Storage 1.4.4 Nanoprobe and Molecular Polymer Storage 1.4.5 Molecular Polymer Storage 1.4.6 Persistent Spectral Holeburning 1.4.7 Coherent Transient Memory 1.4.8 Molecular Storage 1.4.9 All-Optical Magnetic Recording 1.4.10 Electronic Quantum Holography 1.4.11 Scanning Electron Beam Record 1.4.12 3D Integration Solid State Memory 1.4.13 Spintronics Data Storage 1.4.14 Two-Photon 3D Optical Memory 1.4.15 Macromolecular Data Storage 1.4.16 3D Micron Ships Phase-Change Memory 1.4.17 Compositive Application of the Different Principles.. 1.5 Big Data Storage and Application 1.5.1 Cloud Storing 1.5.2 EB-Scale Distributed Storage 1.5.3 Air Traffic Management 1.5.4 Data Exploitation and Communications (DEC) 1.5.5 China Knowledge Resource Integrated Database References2 Mechanism of Multidimensional Optical Storage 2.1 Photophysics and Photochemistry 2.1.1 Light Absorption 2.1.2 Luminescence 2.2 Photoinduced Electron Transfer Process 2.2.1 Emission Lifetime 2.2.2 Ground and Excited State Molecular Interactions 2.2.3 Energy and Electron Transfer 2.3 Other Actions of Photon to Materials 2.3.1 Nonlinear Optical Action 2.3.2 Photoconductive and Photonic Polymers 2.3.3 Photosynthesis 2.3.4 Purple Photosynthetic 2.4 Photophysical Properties of Organometallic Polymers 2.5 Inorganic Photochemistry and Photocatalysis 2.5.1 Electron Storage on ZnO Particles 2.5.2 Particle Size and Absorption 2.5.3 Laser Flash Photolysis 2.5.4 Particle Size and Absorption Threshold 2.5.5 Blue Shift of Absorption upon Illumination 2.5.6 Reducing Reactions and Oxidizing Radicals 2.5.7 Essential Criteria of Photochemical Reactions 2.5.8 Main Types of Photochemical Reactions 2.5.9 Solvents 2.5.10 Direct Sensitized Photolysis 2.6 Reaction Control 2.6.1 Side Reactions Can Easily Become the Major Track . . 2.6.2 Quantum Yield and Chemical Yield 2.6.3 Photochemical Reactions 2.6.4 Alkenes ¡­¡­ 2 Mechanism of Multidimensional Optical Storage3 Recording Materials and Process4 Super Resolution and Laser Sources5 Multi-wavelength and Multi-level (MW/ML) Storage Systems6 Tridimensional (3D) Optical Storage7 Volume Holography and Dynamic Static Speckle Multiplexing8 Muititrack Superposed and Polarized RecordingAppendix A: Constants of Physics and ChemistryAppendix B: Mathematical SymbolsAppendix C: Calculation SymbolsAppendix D: Symbols of Probability AnalysisAppendix E: Symbol of Measurement UniteBibliography